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Abstract

The Pan-Third Pole (PTP) owns complex geography and demographic features where aerosol roles and their impact cannot be neglected as it jeopardizes both the environment and human health. Therefore, we analyzed spatio-temporal aerosol concentration, the influence of meteorological conditions, and underlying aerosol transport mechanisms over the PTP by leveraging observation, satellite dataset, and model outputs. The observation and model simulation result showed that aerosol concentrations exceeded the world health organization (WHO) and China guideline values in most of the locations. This study revealed distinctive seasonality with the highest and lowest aerosol concentrations during the winter and summer seasons, respectively, which could be favored by meteorological conditions and emissions from biomass burning. In response to higher aerosol concentrations, the maximum aerosol optical depth (AOD) values were observed over the major hotspot regions however, interestingly summer high (AOD > 0.8) was observed over the Indo Gangetic Plain (IGP) in South Asia. The columnar aerosol profile indicated that the higher aerosol concentrations were limited within 1–2 km elevation over the densely populated regions over South Asia and Eastern China. However, the significant aerosols concentrations found to be extended as high as 10 km could potentially be driven by the deep convection process and summer monsoon activities. Regionally, the integrated aerosol transport (IAT) for black carbon (BC) and organic carbon (OC) was found to be maximum over SA. Noticeable OC IAT anomaly (~5 times > annual mean) found during spring that was linked with the biomass burning events. Yet, the dust transportation was found to be originated from the arid land and deserts that prolonged especially during summer followed by spring seasons. This study highlights the driver mechanism in aerosol seasonality, transport mechanism, and further motivates the additional assessment into potential dynamic relation between aerosol species, aerosol atmospheric river, and its societal impact.