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Sea2Cloud: from biogenic emission fluxes to cloud properties in the South West Pacific

Urheber*innen

Sellegri,  Karine
External Organizations;

Harvey,  Mike
External Organizations;

Peltola,  Maija
External Organizations;

Saint-Macary,  Alexia
External Organizations;

Barthelmeß,  Theresa
External Organizations;

Rocco,  Manon
External Organizations;

Moore,  Kathryn A.
External Organizations;

Cristi,  Antonia
External Organizations;

Peyrin,  Frederic
External Organizations;

Barr,  Neill
External Organizations;

Labonnote,  Laurent
External Organizations;

Marriner,  Andrew
External Organizations;

McGregor,  John
External Organizations;

Safi,  Karl
External Organizations;

Deppeler,  Stacy
External Organizations;

Archer,  Stephen
External Organizations;

Dunne,  Erin
External Organizations;

Harnwell,  James
External Organizations;

Delanoe,  Julien
External Organizations;

Freney,  Evelyn
External Organizations;

Rose,  Clémence
External Organizations;

Bazantay,  Clément
External Organizations;

Planche,  Céline
External Organizations;

Saiz-Lopez,  Alfonso
External Organizations;

Quintanilla-López,  Jesús E.
External Organizations;

Lebrón-Aguilar,  Rosa
External Organizations;

Rinaldi,  Matteo
External Organizations;

Banson,  Sandra
External Organizations;

Joseph,  Romain
External Organizations;

/persons/resource/236

Lupascu,  Aurelia
IASS Institute for Advanced Sustainability Studies Potsdam;

Jourdan,  Olivier
External Organizations;

Mioche,  Guillaume
External Organizations;

Colomb,  Aurélie
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Olivares,  Gus
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Querel,  Richard
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McDonald,  Adrian
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Plank,  Graeme
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Bukosa,  Beata
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Dillon,  Wayne
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Pelon,  Jacques
External Organizations;

Picard,  David
External Organizations;

Baray,  Jean-Luc
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Tridon,  Frederic
External Organizations;

Donnadieu,  Franck
External Organizations;

Szczap,  Frédéric
External Organizations;

Engel,  Anja
External Organizations;

DeMott,  Paul J.
External Organizations;

Law,  Cliff S.
External Organizations;

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Zitation

Sellegri, K., Harvey, M., Peltola, M., Saint-Macary, A., Barthelmeß, T., Rocco, M., Moore, K. A., Cristi, A., Peyrin, F., Barr, N., Labonnote, L., Marriner, A., McGregor, J., Safi, K., Deppeler, S., Archer, S., Dunne, E., Harnwell, J., Delanoe, J., Freney, E., Rose, C., Bazantay, C., Planche, C., Saiz-Lopez, A., Quintanilla-López, J. E., Lebrón-Aguilar, R., Rinaldi, M., Banson, S., Joseph, R., Lupascu, A., Jourdan, O., Mioche, G., Colomb, A., Olivares, G., Querel, R., McDonald, A., Plank, G., Bukosa, B., Dillon, W., Pelon, J., Picard, D., Baray, J.-L., Tridon, F., Donnadieu, F., Szczap, F., Engel, A., DeMott, P. J., Law, C. S. (2023 online): Sea2Cloud: from biogenic emission fluxes to cloud properties in the South West Pacific. - Bulletin of the American Meteorological Society.
https://doi.org/10.1175/BAMS-D-21-0063.1


Zitierlink: https://publications.rifs-potsdam.de/pubman/item/item_6002766
Zusammenfassung
The goal of the Sea2Cloud project is to study the interplay between surface ocean biogeochemical and physical properties, fluxes to the atmosphere and ultimately their impact on cloud formation under minimal direct anthropogenic influence. Here we present an interdisciplinary approach, combining atmospheric physics and chemistry with marine biogeochemistry, during a voyage between 41 and 47°S in March 2020. In parallel to ambient measurements of atmospheric composition and seawater biogeochemical properties, we describe semi-controlled experiments to characterize nascent sea spray properties and nucleation from gas-phase biogenic emissions. The experimental framework for studying the impact of the predicted evolution of ozone concentration in the Southern Hemisphere is also detailed. After describing the experimental strategy, we present the oceanic and meteorological context including provisional results on atmospheric thermodynamics, composition, and flux measurements. In situ measurements and flux studies were carried out on different biological communities by sampling surface seawater from subantarctic, subtropical and frontal water masses. Air-Sea-Tanks (ASIT) were used to quantify biogenic emissions of trace gases under realistic environmental conditions, with nucleation observed in association with biogenic seawater emissions. Sea spray continuously generated produced sea spray fluxes of 34% of organic matter by mass, of which 4% particles had fluorescent properties, and which size distribution ressembled the one found in clean sectors of the Southern Ocean. The goal of Sea2Cloud is to generate realistic parameterizations of emission flux dependences of trace gases and nucleation precursors, sea spray, cloud condensation nuclei and ice nuclei using seawater biogeochemistry, for implementation in regional atmospheric models.